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비정형 공정부산물 In-Situ 감마선 측정 정확도 향상을 위한효율교정 모델 최적화 방법 개발

Development of an Efficiency Calibration Model Optimization Method for Improving In-Situ Gamma-Ray Measurement for Non-Standard NORM Residues

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초록

In In-situ radioactivity measurement techniques, efficiency calibration models use predefinedmodels to simulate a sample’s geometry and radioactivity distribution. However, simplified efficiencycalibration models lead to uncertainties in the efficiency curves, which in turn affect the radioactivityconcentration results. This study aims to develop an efficiency calibration optimization methodology toimprove the accuracy of in-situ gamma radiation measurements for byproducts from industrial facilities. To accomplish the objective, a drive mechanism for rotational measurement of an byproduct simulatorand a sample was constructed. Using ISOCS, an efficiency calibration model of the designed object wasgenerated. Then, the sensitivity analysis of the efficiency calibration model was performed, and theefficiency curve of the efficiency calibration model was optimized using the sensitivity analysis results. Finally, the radiation concentration of the simulated subject was estimated, compared, and evaluated withthe designed certification value. For the sensitivity assessment of the influencing factors of the efficiencycalibration model, the ISOCS Uncertainty Estimator was used for the horizontal and vertical size anddensity of the measured object. The standard deviation of the measurement efficiency as a function ofthe longitudinal size and density of the efficiency calibration model decreased with increasing energyregion. When using the optimized efficiency calibration model, the measurement efficiency using IUEwas improved compared to the measurement efficiency using ISOCS at the energy of 228Ac (911 keV) forthe nuclide under analysis. Using the ISOCS efficiency calibration method, the difference between themeasured radiation concentration and the design value for each simulated subject measurement directionwas 4.1% (1% to 10%) on average. The difference between the estimated radioactivity concentration andthe design value was 3.6% (1~8%) on average when using the ISOCS IUE efficiency calibration method,which was closer to the design value than the efficiency calibration method using ISOCS. In other words,the estimated radioactivity concentration using the optimized efficiency curve was similar to the designedradioactivity concentration. The results of this study can be utilized as the main basis for the development of regulatory technologies for the treatment and disposal of waste generated during the operation,maintenance, and facility replacement of domestic byproduct generation facilities.

Abstract

In In-situ radioactivity measurement techniques, efficiency calibration models use predefinedmodels to simulate a sample’s geometry and radioactivity distribution. However, simplified efficiencycalibration models lead to uncertainties in the efficiency curves, which in turn affect the radioactivityconcentration results. This study aims to develop an efficiency calibration optimization methodology toimprove the accuracy of in-situ gamma radiation measurements for byproducts from industrial facilities. To accomplish the objective, a drive mechanism for rotational measurement of an byproduct simulatorand a sample was constructed. Using ISOCS, an efficiency calibration model of the designed object wasgenerated. Then, the sensitivity analysis of the efficiency calibration model was performed, and theefficiency curve of the efficiency calibration model was optimized using the sensitivity analysis results. Finally, the radiation concentration of the simulated subject was estimated, compared, and evaluated withthe designed certification value. For the sensitivity assessment of the influencing factors of the efficiencycalibration model, the ISOCS Uncertainty Estimator was used for the horizontal and vertical size anddensity of the measured object. The standard deviation of the measurement efficiency as a function ofthe longitudinal size and density of the efficiency calibration model decreased with increasing energyregion. When using the optimized efficiency calibration model, the measurement efficiency using IUEwas improved compared to the measurement efficiency using ISOCS at the energy of 228Ac (911 keV) forthe nuclide under analysis. Using the ISOCS efficiency calibration method, the difference between themeasured radiation concentration and the design value for each simulated subject measurement directionwas 4.1% (1% to 10%) on average. The difference between the estimated radioactivity concentration andthe design value was 3.6% (1~8%) on average when using the ISOCS IUE efficiency calibration method,which was closer to the design value than the efficiency calibration method using ISOCS. In other words,the estimated radioactivity concentration using the optimized efficiency curve was similar to the designedradioactivity concentration. The results of this study can be utilized as the main basis for the development of regulatory technologies for the treatment and disposal of waste generated during the operation,maintenance, and facility replacement of domestic byproduct generation facilities.

참고문헌 (20)

  1. Radiation Protection and Management of NORM Residues in the Phosphate Industry, "IAEA", IAEA, ~, pp.IAEA Safety Reports Series No.78 (2013)
  2. Radiation Protection and NORM Residue Management in the Titanium Dioxide and Related Industries, "IAEA", IAEA, ~, pp.IAEA Safety Reports Series No.76 (2012)
  3. Mueller WF, "In-situ Measurements and Analysis of Naturally Occurring Radioactive Materials", ANIMMA Conference (2013)
  4. Frosio T, "A new gamma spectroscopy methodology based on probabilistic uncertainty estimation and conservative approach", Appl. Radiat. Isot, 155, pp.108929~ (2020)
  5. Bosko A, "Efficiency Optimization Employing Random and Smart Search Using Multiple Counts and Line Activity Consistency Benchmarks", Proceedings of the 37th Waste Management Symposia, Phoenix (2011)
  6. Bourva L, "Probabilistic uncertainty estimator for gamma-spectroscopy measurements", J. Radioanal. Nucl. Chem, 276, pp.589~594 (2008)[DOI]
  7. IAEA., "Naturally Occurring Radioactive Material (NORM VII)", Proceedings of an International Symposium (2013)
  8. Hong SB, "Evaluation of residual radioactivity in buildings using ISOCS", Proceedings of the Korean Radioactive Waste Society Conference, 5, pp.55~56 (2008)
  9. 정현철, "In-Situ 측정법을 이용한 고리 원자로 방사선원항 평가", Journal of Nuclear Fuel Cycle and Waste Technology, 12(2), pp.171~178 (2014), 한국방사성폐기물학회[DOI]
  10. Choi JG, "ISOCS V4.2 Calibration Software User Interface", ~ (2015)
  11. Development of safety management technology for decommissioning of industrial facilities generating large scale NORM residues, "KINS.", KINS, ~, pp.KINS (2017), HR-1631
  12. Development of technical guidelines and work procedures for treatment and disposal of NORM Residues based on field test, "KINS.", KINS, ~, pp.KINS (2016), HR-1519
  13. Development of radiological safety evaluation methods for industry using monazite and other naturally occurring radioactive materials, "KINS", KINS, ~, pp.KINS (2016), HR-1456
  14. IAEA, "RS_RGTh-1 Reference sheet", ~
  15. Canberra, "Advanced ISCOS Measurement"Using the ISOCS Uncertainty Estimator"", ISOSC manual SU-476-3, ~ (2018)
  16. F. Bronson, "Probabilistic uncertainty estimator for gamma-spectroscopy measurements", Journal of Radioanalytical and Nuclear Chemistry, 276(3), pp.589~594 (2008), Springer Science and Business Media LLC[DOI]
  17. Measurement of radioactivity in the environment, Part 3: Test method of gamma-emitting radionuclides using gammaray spectrometry, "ISO", ISO, ~, pp.ISO 18589-3 (2015)
  18. Radwaste Drum Assay Technology by Segmented Gamma Scanning System, "KAERI", KAERI, ~, pp.KAERI (2009), TR-3711[DOI]
  19. Mirion Technologies, "Model S573 ISOCS Calibration Software", ~ (2013)
  20. In Situ Gamma Spectroscopy with ISOCSTM, "Mirion Technologies", An In-Situ Object Counting System, ~ (2008)

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