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Feasibility study of a resistive-type sodium aerosol detector with ZnO nanowires for sodium-cooled fast reactors

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초록

In sodium systems, leakage is one of the safety concerns; it can cause chemical reactions, which may result in fires. There are contact and non-contact types of leak detectors, and the conventional method of non-contact type detection is by gas sampling. Because of the complexity of this method, there has always been a need for a simple gas sensor, and the resistive-type nanostructure ZnO sensor is a promising option with various advantages. In this study, a ZnO sensor was fabricated, and the concept was tested as a leak detector using a dedicated experiment facility. The experiment results showed distinctive changes in resistance with the presence of sodium aerosol under various conditions. Replacing the conventional gas sampling with the ZnO sensors is expected to enable identification of the leakage location if used as a point-wise instrumentation and to greatly reduce the total cost, making the system simple, light, and effective. For further study, more tests will be performed to evaluate the sensitivity of key parameters under various conditions

Abstract

In sodium systems, leakage is one of the safety concerns; it can cause chemical reactions, which may result in fires. There are contact and non-contact types of leak detectors, and the conventional method of non-contact type detection is by gas sampling. Because of the complexity of this method, there has always been a need for a simple gas sensor, and the resistive-type nanostructure ZnO sensor is a promising option with various advantages. In this study, a ZnO sensor was fabricated, and the concept was tested as a leak detector using a dedicated experiment facility. The experiment results showed distinctive changes in resistance with the presence of sodium aerosol under various conditions. Replacing the conventional gas sampling with the ZnO sensors is expected to enable identification of the leakage location if used as a point-wise instrumentation and to greatly reduce the total cost, making the system simple, light, and effective. For further study, more tests will be performed to evaluate the sensitivity of key parameters under various conditions

참고문헌 (13)

  1. Sujatha Pavan Narayanam, "Theoretical simulation on evolution of suspended sodium combustion aerosols characteristics in a closed chamber", Nuclear Engineering and Technology, 54(6), pp.2077~2083 (2022), 한국원자력학회[DOI]
  2. S. P. Narayanam, "Experimental measurements and theoretical simulation of sodium combustion aerosol leakage through capillaries", Prog. Nucl. Energy, 118, pp.103111~ (2020)
  3. V. Subramanian, "Studies on sodium aerosols dispersion in open environment for fast reactor safety", Ann. Nucl. Energy, 125, pp.63~73 (2019)
  4. 유재운, "Overall System Description and Safety Characteristics of Prototype Gen IV Sodium Cooled Fast Reactor in Korea", Nuclear Engineering and Technology, 48(5), pp.1059~1070 (2016), 한국원자력학회
  5. 이제환, "Design of large-scale sodium thermal-hydraulic integral effect test facility, STELLA-2", Nuclear Engineering and Technology, 54(9), pp.3551~3566 (2022), 한국원자력학회[DOI]
  6. N. -i. Tak, "Improvement of GAMMAþcode for system transient and thermo-fluid safety analysis of sodium-cooled fast reactors", Nucl. Eng. Des, 399, pp.112002~ (2022)
  7. G. Vijayakumar, "Performance evaluation of PFBR wire type sodium leak detectors", Nucl. Eng. Des, 241, pp.2271~2279 (2011)
  8. J. I. Sylvi, "Development of sodium leak detectors for PFBR", Nucl. Eng. Des, 249, pp.419~431 (2012)
  9. H. Yamamoto, "Development of fluctuation monitor type sodium ionization detector", J. Nucl. Sci. Technol, 23, pp.573~581 (1986)
  10. T. Aoyama, "Development of sodium leak detection technology using laser resonance ionization mass spectrometry", J. Nucl. Sci. Technol, 45, pp.43~50 (2008)
  11. Cecile Maury, "Analysis of liquid sodium purity by laser-induced breakdown spectroscopy. Modeling and correction of signal fluctuation prior to quantitation of trace elements", Spectroc. Acta Pt. B Atom. Spectr, 82, pp.28~35 (2013)
  12. L. Zhu, "Room-temperature gas sensing of ZnO-based gas sensor : a review", Sens. Actuator B Chem, 267, pp.242~261 (2017)
  13. B. Gong, "UV irradiationassisted ethanol detection operated by the gas sensor based on ZnO nanowires", optical fiber hybrid structure, 2017, pp.245, 821~827

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