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Database of virtual spectrum of artificial radionuclides for education and training in in-situ gamma spectrometry

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주제분류원자력공학

초록

As the field of application of in-situ gamma spectroscopy is diversified, proficiency is required for consistent and accurate analysis. In this study, a program was developed to virtually create gamma energy spectra of artificial nuclides, which are difficult to obtain through actual measurements, for training. The virtual spectrum was created by synthesizing the spectra of the background radiation obtained through actual measurement and the theoretical spectra of the artificial radionuclides obtained by a Monte Carlo simulation. Since the theoretical spectrum can only be obtained for a given geometrical structure, representative major geometries for in-situ measurement (ground surface, concrete wall, radioactive waste drum) and the detectors (HPGe, NaI(Tl), LaBr3(Ce)) were predetermined. Generated virtual spectra were verified in terms of validity and harmonization by gamma spectrometry and energy calibration. As a result, it was confirmed that the energy calibration results including the peaks of the measured spectrum and the peaks of the theoretical spectrum showed differences of less than 1 keV from the actual energies, and that the calculated radioactivity showed a difference within 20% from the actual inputted radioactivity. The verified data were assembled into a database and a program that can generate a virtual spectrum of desired condition was developed

Abstract

As the field of application of in-situ gamma spectroscopy is diversified, proficiency is required for consistent and accurate analysis. In this study, a program was developed to virtually create gamma energy spectra of artificial nuclides, which are difficult to obtain through actual measurements, for training. The virtual spectrum was created by synthesizing the spectra of the background radiation obtained through actual measurement and the theoretical spectra of the artificial radionuclides obtained by a Monte Carlo simulation. Since the theoretical spectrum can only be obtained for a given geometrical structure, representative major geometries for in-situ measurement (ground surface, concrete wall, radioactive waste drum) and the detectors (HPGe, NaI(Tl), LaBr3(Ce)) were predetermined. Generated virtual spectra were verified in terms of validity and harmonization by gamma spectrometry and energy calibration. As a result, it was confirmed that the energy calibration results including the peaks of the measured spectrum and the peaks of the theoretical spectrum showed differences of less than 1 keV from the actual energies, and that the calculated radioactivity showed a difference within 20% from the actual inputted radioactivity. The verified data were assembled into a database and a program that can generate a virtual spectrum of desired condition was developed

참고문헌 (12)

  1. J. Kluson, "Environmental monitoring and in situ gamma spectrometry", Radiat. Phys. Chem, 61, pp.209~216 (2001)
  2. 홍상범, "Application of In Situ Measurement for Site Remediation and Final Status Survey of Decommissioning KRR Site", 방사선방어학회지, 41(2), pp.173~178 (2016), 테스트학회[DOI]
  3. B. Lee, "Radiological analysis for radioactivity depth distribution in activated concrete using gamma-ray spectrometry", Appl. Radiat. Isot, 169, pp.109558~ (2021)
  4. N. K. S¸ ahin, "A review of the nationwide proficiency test on natural radioactivity measurements by gamma spectrometry", Appl. Radiat. Isot, 109, pp.49~53 (2016)
  5. O. El Samad, "Proficiency tests : a tool for improvement and testing analytical performance at Gamma-Ray Spectroscopy Laboratory", Accred Qual. Assur, 26, pp.121~127 (2021)
  6. Gamma-Ray Spectrometry in the Environment, vols. 15-27, "International Commission on Radiation Units and Measurements", ICRU, ~, pp.Report 53 (1994)
  7. International Organization for Standardization, "Measurement of Radioactivity in the Environment e Soil e Part 7: in Situ Measurement of Gamma-Emitting Radionuclides", ISO 18589-7, ~ (2013)
  8. Managing Low Radioactivity Material from the Decommissioning of Nuclear Facilities, "International Atomic Energy Agency", ~, pp.Technical reports series No. 462 (2008)
  9. Y. Y. Ji, "Development of the environmental radiation survey program and its application to in situ gamma-ray spectrometry", Health Phys, 116, pp.840~851 (2019)
  10. Y. Y. Ji, "Development and performance of a multipurpose system for the environmental radiation survey based on a LaBr3(Ce)detector", IEEE Trans. Nucl. Sci, 66, pp.2422~2429 (2019)
  11. MIRION tech, "in Situ Gamma Spectroscopy with ISOCSTM, an in Situ Object Counting System", M2352-11, ~ (2008)
  12. H. Cheng, "Intrinsic background radiation of LaBr3(Ce)detector via coincidence measurements and simulations", Nucl. Sci. Tech, 31, pp.99~ (2020)

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