Aerodynamic Particle Sizer (APS)를 이용한 고농도 PM10 사례 중 황사 판별기법 개발
Developing a Method for Detecting the Asian dust event Among High PM10 events Using Aerodynamic Particle Sizer (APS)
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초록
Log normalized volume size distribution (dV/dlogDp) with 52 size ranges from 0.5 to 20.0 μm was measured for the cases of high PM10 mass concentration (> 200 μg m-³) using the Aerodynamic Particle Sizer (APS) at the Korea Global Atmosphere Watch Center (KGAWC) from 6 April, 2006 to 5 April, 2007. Black Carbon (BC), gaseous pollutants of NOX and SO₂, and Ångstrom exponent were also measured to examine the properties of the volume size distribution. From distinct difference of the high volume concentration (> 100 μm³ cm-³), the volume size distribution for each event day was classified into four types: (1) Type 1 had the high volume concentration for supermicron particles from 2.3 to 6.0 μm and maximum average volume concentration was 160.7 μm³ cm-³ at 3.5 μm. (2) Type 2 represented the high volume concentration in the both size range of submicron (0.7–1.0 μm) and supermicron particles (2.1–4.1 μm) and similar maxima of 126.1 μm³ cm-³ and 136.2 μm³ cm-³ were found at 0.8 and 3.3 μm respectively. (3) Type 3 showed the high volume concentration in the size range of 0.5–3.5 μm and highest volume concentration of 201.1 μm³ cm-³ at the particle size bin of 0.8 μm. (4) Type 4 was characterized by the high volume concentration for the fine particles less than 1.2 μm and very high concentration of 446.8 μm³ cm-³. Ångstrom exponent, concentration of gaseous (NOX and SO2), and particle (BC) pollutants suggested that Type 1 was a typical volume size distribution for the Asian dust and Type 3 provided transportation of air pollutants. The distribution in Type 2 found to have both characteristics of the Asian dust and air pollutants, and Type 4 was took place during the foggy atmosphere containing high density of local pollutants. Based on the properties of volume size distribution, we can identify the three major events contributing the increase of PM10 mass concentration, and hope to provide a guideline for discriminating the Asian dust from high PM10 events. More case studies and longer measurements provide a data set to advance this determination method.
Abstract
Log normalized volume size distribution (dV/dlogDp) with 52 size ranges from 0.5 to 20.0 μm was measured for the cases of high PM10 mass concentration (> 200 μg m-³) using the Aerodynamic Particle Sizer (APS) at the Korea Global Atmosphere Watch Center (KGAWC) from 6 April, 2006 to 5 April, 2007. Black Carbon (BC), gaseous pollutants of NOX and SO₂, and Ångstrom exponent were also measured to examine the properties of the volume size distribution. From distinct difference of the high volume concentration (> 100 μm³ cm-³), the volume size distribution for each event day was classified into four types: (1) Type 1 had the high volume concentration for supermicron particles from 2.3 to 6.0 μm and maximum average volume concentration was 160.7 μm³ cm-³ at 3.5 μm. (2) Type 2 represented the high volume concentration in the both size range of submicron (0.7–1.0 μm) and supermicron particles (2.1–4.1 μm) and similar maxima of 126.1 μm³ cm-³ and 136.2 μm³ cm-³ were found at 0.8 and 3.3 μm respectively. (3) Type 3 showed the high volume concentration in the size range of 0.5–3.5 μm and highest volume concentration of 201.1 μm³ cm-³ at the particle size bin of 0.8 μm. (4) Type 4 was characterized by the high volume concentration for the fine particles less than 1.2 μm and very high concentration of 446.8 μm³ cm-³. Ångstrom exponent, concentration of gaseous (NOX and SO2), and particle (BC) pollutants suggested that Type 1 was a typical volume size distribution for the Asian dust and Type 3 provided transportation of air pollutants. The distribution in Type 2 found to have both characteristics of the Asian dust and air pollutants, and Type 4 was took place during the foggy atmosphere containing high density of local pollutants. Based on the properties of volume size distribution, we can identify the three major events contributing the increase of PM10 mass concentration, and hope to provide a guideline for discriminating the Asian dust from high PM10 events. More case studies and longer measurements provide a data set to advance this determination method.
참고문헌 (17)
- 지구대기감시보고서 2005, "기상청", 기상청, 125~ (2006)
- 이영곤, "지구대기감시센터에서 Aerodynamic Particle Sizer (APS)를 이용한 고농도 PM10 사례분석", 한국입자에어로졸학회 학술대회, pp.45~46 (2007)
- Anderson, "Aerosol backscattering fraction and single scattering albedo: Measured values and uncertainties at a coastal station in the Pacific Northwest", J. Geophys. Res., 106(D18), pp.20767~20782 (1999)
- Bates, T. S., "Regional physical and chemical properties of the marine boundary layer aerosol across the Atlantic during Aerosol99: An overview", J. Geophys. Res., 106(D18), pp.20767~20782 (2001)
- Bates, T. S., "Regional marine boundary layer aerosol size distributions in the Indian, Atlantic, and Pacific Oceans: A comparison of INDOEX measurements with ACE-1, CE-2, and Aerosol99", J. Geophys. Res., 107(D19), pp.8026~ (2002)[DOI]
- Bates, T. S., "Marine boundary layer dust and pollutant transport associated with the passage of a frontal system over eastern Asia", J. Geophys. Res., 109(D19), pp.S19~ (2004)[DOI]
- Asian transport of aerosols to Mauna Loa Observatory, Spring 1994, "Cahill, T. A.", Climate Monitoring and Diagnostics Laboratory, 114~116, pp.Summary Report 1994–1995, No. 23 (1995)
- Darmenova, K., "Characterization of east Asian dust outbreaks in the spring of 2001 using ground-based and satellite data", J. Geophys. Res., 110, pp.D02204~ (2001)[DOI]
- Hobbs, P. V., "Introduction to atmospheric chemistry", pp.262~ (2000), Cambridge Univ. Press
- Jaffe, D., "The 2001 Asian Dust Events: Transport and Impact on Surface Aerosol Concentrations in the U.S.", Eos, Transactions, American Geophysical Union, 84(46), pp.501~516 (2001)
- Lee, Y. G., "Design and install of the integrated aerosol inlet in the KGAWO", Autumn Conference of the Korean Meteorological Society, pp.456~457 (2005)
- Liou, K., "An Introduction to Atmospheric Radiation, International Geophysics Series, No. 84", pp.583~ (2002), Academic Press
- Sokolik, I. N., "Introduction to special section on mineral dust: Outstanding problems in quantifying the radiative impact of mineral dust", J. Geophys. Res., 106(18), pp.18015~18028 (2001)
- Un, J., "Spatial and temporal characteristics of dust storms in China and its surrounding regions, 1960 - 1999: Relations to source area and climate", J. Geophys. Res., 106, pp.10325~10333 (1999)
- Uno, I., "Numerical study of Asian dust transport during the springtime of 2001 simulated with the Chemical Weather Forecasting System (CFORS) model", J. Geophys. Res., 109(D19), pp.S24~ (2001)[DOI]
- Wang, J., "Clear-column radiative closure during ACE-Asia: Comparison of multiwavelength extinction derived from particle size and composition with results from Sun photometry", J. Geophys. Res., 107(D23) (2002)[DOI]
- Zhou, J., "Lidar observations of Asian dust over Hefei, China, in spring 2000", J. Geophys. Res., 107(D15), pp.4252~ (2000)[DOI]
