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공기 궤 유입경로에 따른 한반도 서울 상공의 전체 및 유기 에어로졸 농도 변화 분석

Dependence of Total and Carbonaceous Aerosol Concentrations on Transport Pathways in Seoul, Korea

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주제분류대기과학

초록

Recently increased anthropogenic aerosols change the radiative energy balance andaffect human life. The management of air quality requires monitoring both the local emissionsand transported pollutants. In order to estimate the quantitative contribution of long-rangetransport from remote sources on aerosol concentrations in Seoul, the airmasses were classifiedinto five types with respect to their pathways. When airmass came from west over strongemission regions in China, high concentrations of PM10, PM2.5, black carbon (BC), organic carbon(OC), and elemental carbon (EC) were found, even higher than those for the stagnated airmass. High OC concentrations were found when airmass came from north while BC, EC, andPM2.5 concentrations were lower than those of the stagnated airmasses. During dust events, thePM2.5 and PM10 concentrations increased significantly while carbonaceous aerosol concentrationsdid not increased. The temporal variations of aerosol concentrations in Seoul wereaffected by the seasonal variations of airmass pathways. The high PM2.5 concentrations over100 μg m−3 appeared most frequently when the airmasses came from west.

Abstract

Recently increased anthropogenic aerosols change the radiative energy balance andaffect human life. The management of air quality requires monitoring both the local emissionsand transported pollutants. In order to estimate the quantitative contribution of long-rangetransport from remote sources on aerosol concentrations in Seoul, the airmasses were classifiedinto five types with respect to their pathways. When airmass came from west over strongemission regions in China, high concentrations of PM10, PM2.5, black carbon (BC), organic carbon(OC), and elemental carbon (EC) were found, even higher than those for the stagnated airmass. High OC concentrations were found when airmass came from north while BC, EC, andPM2.5 concentrations were lower than those of the stagnated airmasses. During dust events, thePM2.5 and PM10 concentrations increased significantly while carbonaceous aerosol concentrationsdid not increased. The temporal variations of aerosol concentrations in Seoul wereaffected by the seasonal variations of airmass pathways. The high PM2.5 concentrations over100 μg m−3 appeared most frequently when the airmasses came from west.

참고문헌 (23)

  1. Birch, M. E., "Elemental carbonbased method for monitoring occupational exposures to particulate diesel exhaust", Aerosol Sci. Technol, 25, pp.221~241 (1996)
  2. Cheng, Y. H., "Comparison of the TSI model 8520 and Grimm Series 1. 108 portable aerosol instruments used to monitor particulate matter in an iron foundry", J. Occup. Environ. Hyg, 5, pp.157~168 (2008)
  3. Cheng, Y. H., "Measurement of particle mass concentrations and size distributions in an underground station", Aerosol Air Qual Res, 10, pp.22~29 (2010)
  4. Hansen, A. D. A., "The aethalometer-an instrument for the real-time measurement of optical-absorption by aerosol-particles", Sci. Total Environ, 36, pp.191~196 (1984)
  5. He, Z., "Characteristics of PM2. 5 species and long-range transport of air masses at Taean background station, South Korea", Atmos. Environ, 37, pp.219~230 (2003)
  6. Heo, J. B., "Source apportionment of PM2. 5 in Seoul, Korea", Atmos. Chem. Phys, 9, pp.4957~4971 (2009)
  7. Hwang, I., "Estimation of source apportionment and potential source locations Of PM2. 5 at a west coastal IMPROVE site", Atmos. Environ, 41, pp.506~518 (2007)
  8. Jeong, C. H., "Measurement of real-time PM2. 5 mass, sulfate, and carbonaceous aerosols at the multiple monitoring sites", Atmos. Environ, 38, pp.5247~5256 (2004)
  9. Jeong, J. I., "Source contributions to carbonaceous aerosol concentrations in Korea", Atmos. Environ, 45, pp.1116~1125 (2011)
  10. Jeong, U., "Determination of the inter-annual and spatial characteristics of the contribution of longrange transport to SO2 levels in Seoul between 2001 and 2010 based on conditional potential source contribution function(CPSCF)", Atmos. Environ, 70, pp.307~317 (2013)
  11. Jeong, U., "Estimation of the contributions of long range transported aerosol in East Asia to carbonaceous aerosol and PM concentrations in Seoul, Korea using highly time resolved measurements : a PSCF model approach", J. Environ. Monitor, 13, pp.1905~1918 (2011)
  12. Kim, Y. J., "Investigation of carbon pollution episodes using semicontinuous instrument in Incheon, Korea", Atmos. Environ, 40, pp.4064~4075 (2006)
  13. Moy, L. A., "Relationship between back trajectories and tropospheric trace gas concentrations in rural Virginia", Atmos. Environ, 28, pp.2789~2800 (1994)
  14. Polidori, A., "Local and regional secondary organic aerosol : Insights from a year of semi-continuous carbon measurements at Pittsburgh", Aerosol Sci. Technol, 40, pp.861~872 (2006)
  15. Pope, C. A., "Lung cancer, cardiopulmonary mortality, and long-term exposure to fine particulate air pollution", J. Amer. Med. Assoc, 287, pp.1132~1141 (2002)
  16. Ramanathan, V., "Atmosphere-Aerosols, climate, and the hydrological cycle", Science, 294, pp.2119~2124 (2001)
  17. Schmid, O., "Spectral light absorption by ambient aerosols influenced by biomass burning in the Amazon Basin. I : Comparison and field calibration of absorption measurement techniques", Atmos. Chem. Phys, 6, pp.3443~3462 (2006)
  18. Seinfeld, J. H., "Atmospheric chemistry and physics from air pollution to climate change" (2006), Wiley
  19. Stohl, A., "Computation, accuracy and applications of trajectories-A review and bibliography", Atmos.Environ., 32, pp.947~966 (1998)
  20. Wang, J., "Intercomparison between satellite-derived aerosol optical thickness and PM2.5 mass: Implications for air quality studies", Geophys. Res. Lett, 30 (2003)
  21. Watson, J. G., "Visibility : Science and regulation", J. Air Waste Manage, 52, pp.628~713 (2002)
  22. Weingartner, E., "Absorption of light by soot particles : determination of the absorption coefficient by means of aethalometers", J. Aerosol Sci, 34, pp.1445~1463 (2003)
  23. "HYSPLIT4.8 (HYbrid Single-Particle Lagrangian Integrated Trajectory) Model" (2008)[URL]

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