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Effect of annealing atmosphere on defects, light absorption and imprinting properties of Bi4Ti3O12 films

Lingxu Wang|Huiying Liu|Liqiang Liu|Fengqing Zhang
청정에너지연구소 (Clean-Energy Research Institute)|2021.02|Journal of Ceramic Processing Research|제22권 제1호|pp. 121-129|DOI 10.36410/jcpr.2021.22.1.121

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참고문헌

키워드

AgingBi vacanciesLight absorptionImprinting
주제분류재료공학

초록

In order to studying the effect of the annealing atmospheres (nitrogen and air) on the films, two kinds of Bi4Ti3O12 (BIT) samples were prepared by the sol-gel and layer-by-layer thermal annealing method. Various factors, including lesser VO••, more V'B'i and greater grain size in the air-annealed samples, interacted on the ferroelectric and light absorption properties. However, more (V'B'i)-(VO••) reinforced the imbalance of electron capture in the ITO/BIT/Au capacitors, resulting in stronger imprinting. And the arrangement of (V'B'i)-(VO••) and the domain pinning in the air-annealed films resulted in more serious aging effect.

Abstract

In order to studying the effect of the annealing atmospheres (nitrogen and air) on the films, two kinds of Bi4Ti3O12 (BIT) samples were prepared by the sol-gel and layer-by-layer thermal annealing method. Various factors, including lesser VO••, more V'B'i and greater grain size in the air-annealed samples, interacted on the ferroelectric and light absorption properties. However, more (V'B'i)-(VO••) reinforced the imbalance of electron capture in the ITO/BIT/Au capacitors, resulting in stronger imprinting. And the arrangement of (V'B'i)-(VO••) and the domain pinning in the air-annealed films resulted in more serious aging effect.

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