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Measurement of deuterium concentration in heavy water utilizing prompt gamma neutron activation analysis (PGNAA) in comparison with MCNPX simulation results

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주제분류원자력공학

초록

Considering the importance of deuterium in nuclear science including medical and industrial researches such as (BNCT) and nuclear reactors respectively, it is important to study various possible ways in addition to common methods for measuring its concentration. This study is an effort to measure deuterium concentration using PGNAA. The main idea is to calculate the area under 2.23 MeV gammarays photo peak resulting from neutron collision with Hydrogen atoms which are in mix with deuterium in samples. The study carried out by both simulation and experiment. Monte Carlo MCNPX2.6 code has been used for simulation and based on its acceptable results an experimental setup has been arranged. The coordination of results was in the range of R ¼ 0.99 and R ¼ 0.98 in simulation and experiment respectively. The accuracy of the study has been investigated by measuring the concentration of an unknown sample by both PGNAA and Fourier transform infrared spectroscopy (FT-IR) methods in which there were acceptable correlation between these two methods.

Abstract

Considering the importance of deuterium in nuclear science including medical and industrial researches such as (BNCT) and nuclear reactors respectively, it is important to study various possible ways in addition to common methods for measuring its concentration. This study is an effort to measure deuterium concentration using PGNAA. The main idea is to calculate the area under 2.23 MeV gammarays photo peak resulting from neutron collision with Hydrogen atoms which are in mix with deuterium in samples. The study carried out by both simulation and experiment. Monte Carlo MCNPX2.6 code has been used for simulation and based on its acceptable results an experimental setup has been arranged. The coordination of results was in the range of R ¼ 0.99 and R ¼ 0.98 in simulation and experiment respectively. The accuracy of the study has been investigated by measuring the concentration of an unknown sample by both PGNAA and Fourier transform infrared spectroscopy (FT-IR) methods in which there were acceptable correlation between these two methods.

참고문헌 (11)

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  3. M. N. Nasrabadi, "Critical heavy water level and some parameters for the HWZPR reactor core using MCNP4c code", Annals of Nuclear Energy, 73, pp.496~499 (2014)
  4. D. L. Chichester, "Measurement of nitrogen in the body using a commercial PGNAA systemdphantom experiments", Applied Radiation and Isotopes, 60(1), pp.55~61 (2004)
  5. M.D. Glascock, "An Overview of Neutron Activation Analysis", World Wide Web, ~ (2004)
  6. S. F. Masoudi, "BNCT of skin tumors using the highenergy DT neutrons", Applied Radiation and Isotopes, 122, pp.158~163 (2017)
  7. Development of a BNCT Facility Based on Axial DeuteriumeDeuterium (DeD) Neutron Generator Using MCNP Code, "K. Bergaoui", IAEA, ~ (2017)
  8. S. A. Wallace, "The influence of heavy water on boron requirements for neutron capture therapy", Medical Physics, 22(5), pp.585~590 (1995)
  9. J. R. Lamarsh, "Introduction to nuclear engineering. Upper saddle river" (2001), Prentice hall
  10. L. Taghizadeh, "Comparison of probabilistic and deterministic methods for calculation of kinetic parameters of HWZPR", Annals of Nuclear Energy, 165, pp.108633~ (2022)
  11. Zahra Nasrazadani, "Investigating Dynamic Parameters in HWZPR Based on the Experimental and Calculated Results", Nuclear Engineering and Technology, 48(5), pp.1120~1125 (2016), 한국원자력학회

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