본문 바로가기
KERD
논문KCI 등재

서울의 일차탄소성분 입자 농도 변화 및 관리 방향

Trend and policy directions of primary carbonaceous aerosols in Seoul

0

조회

0

다운로드

0

인용

0

참고문헌

키워드

초록

The concentrations of polycyclic aromatic hydrocarbons (PAHs) and elemental carbon (EC) in particulate matter, typical primary aerosols have decreased in Seoul between 2003 and 2018 (80% for PAHs and 85% for EC). The yearly mean benzo[a]pyrene (BaP) concentration has been lower than 1 ng/m3 since 2010-2011, the target value set by the European Union (EU) and China. A series of policies related to solid fuel and vehicle in South Korea and China should be effective in the reduction of the ambient PAHs and EC concentrations. But the emission data of PAHs and EC at both countries did not support that hypothesis. Possible causes are uncertainties in the emission inventories of primary carbonaceous aerosols in South Korea and China, although there may be a minor effect of the emissions from North Korea on the concentrations in Seoul. Thus the further policy directions against PAHs and EC such as improvements of emissions inventories and measurements, intensive regulation of non-road mobile sources and control of PAHs derivatives are discussed.

Abstract

The concentrations of polycyclic aromatic hydrocarbons (PAHs) and elemental carbon (EC) in particulate matter, typical primary aerosols have decreased in Seoul between 2003 and 2018 (80% for PAHs and 85% for EC). The yearly mean benzo[a]pyrene (BaP) concentration has been lower than 1 ng/m3 since 2010-2011, the target value set by the European Union (EU) and China. A series of policies related to solid fuel and vehicle in South Korea and China should be effective in the reduction of the ambient PAHs and EC concentrations. But the emission data of PAHs and EC at both countries did not support that hypothesis. Possible causes are uncertainties in the emission inventories of primary carbonaceous aerosols in South Korea and China, although there may be a minor effect of the emissions from North Korea on the concentrations in Seoul. Thus the further policy directions against PAHs and EC such as improvements of emissions inventories and measurements, intensive regulation of non-road mobile sources and control of PAHs derivatives are discussed.

참고문헌 (32)

  1. "(CIS/97/00215)" (1995)[URL]
  2. Bae, M., "PM2.5 Simulations for the Seoul Metropolitan Area:(V) Estimation of North Korean Emission Contribution", Journal of Korean Society for Atmospheric Environment, 34(2) (2018)[DOI]
  3. Cheng, Y., "Decreasing concentrations of carbonaceous aerosols in China from 2003 to 2013", Scientific Reports, 11(1), pp.5352~ (2021)[DOI]
  4. Cheong S. W., "Effects and Management Risk of Air Quality Management Policies in the Seoul Metropolitan Area: Focusing on lessening PM10 and NO2 in the pollution reduction project of in-use diesel vehicles", Cheong, Sang Woo, Kim, Nan Young, 37, pp.5~36 (2021)[DOI]
  5. Choi, E. L., "Long-term(1993-2018)particulate polycyclic aromatic hydrocarbons(PAHs)concentration trend in the atmosphere of Seoul : Changes in major sources and health effects", Atmospheric Environment, 319, pp.120418~ (2024)[DOI]
  6. Choi, N. R., "Speciation and source identification of organic compounds in PM10 over Seoul, South Korea", Chemosphere, 144, pp.1589~1596 (2016)[DOI]
  7. Crippa, M., "High resolution temporal profiles in the Emissions Database for Global Atmospheric Research", Scientific Data, 7(1), pp.121~ (2020)[DOI]
  8. "Directive 2004/107/EC of the European Parliament and of the Council of 15 December 2004 relating to arsenic, cadmium, mercury, nickel and polycyclic aromatic hydrocarbons in ambient air" (2004)[URL]
  9. Han, H., "Evaluation of the Effectiveness and Efficiency of Atmospheric Particulates Reduction Policy : The Case of South Korea", Asian Journal of Atmospheric Environment, 16(2), pp.2021130~ (2023)[DOI]
  10. Han, S., "Temporal Trend of the Major Contributors for the Particulate Polycyclic Aromatic Hydrocarbons(PAHs)in Seoul", Aerosol and Air Quality Research, 19(2), pp.318~330 (2019)[DOI]
  11. Hayakawa, K., "Long-Term Trends in Urban Atmospheric Polycyclic Aromatic Hydrocarbons and Nitropolycyclic Aromatic Hydrocarbons : China, Russia, and Korea from 1999 to 2014", International journal of environmental research and public health, 17(2), pp.431~ (2020)[DOI]
  12. "Speciated atmospheric mercury on haze and non-haze days in an inland city in China" (2016)[URL]
  13. Hong, S. B., "PAHs concentrations of PM10 in Seoul metropolitan area(in Korean)", Journal of Korean Society for Atmospheric Environment, 25(4), pp.347~359 (2009)[DOI]
  14. Kang, M., "Recent Occurrence of PAHs and n-Alkanes in PM2.5 in Seoul, Korea and Characteristics of their Sources and Toxicity", Int J Environ Res Public Health, 17(4) (2020)[DOI]
  15. Kim, B. M., "A multivariate receptor modeling study of air-borne particulate PAHs : Regional contributions in a roadside environment", Chemosphere, 144, pp.1270~1279 (2016)[DOI]
  16. Kim, I. S., "Impact of polycyclic aromatic hydrocarbon(PAH)emissions from North Korea to the air quality in the Seoul Metropolitan Area, South Korea", Atmospheric Environment, 70, pp.159~165 (2013)[DOI]
  17. Kim, Y., "Fifteen-year trends in carbon species and PM2. 5 in Seoul, South Korea(2003–2017)", Chemosphere, 261, pp.127750~ (2020)[DOI]
  18. Kim, Y. P., "Trend of Air Quality in Seoul : Policy and Science", Aerosol and Air Quality Research, 18(9), pp.2141~2156 (2018)[DOI]
  19. Lee, J. Y., "Source apportionment of the particulate PAHs at Seoul, Korea: impact of long range transport to a megacity", Atmos. Chem. Phys., 7(13), pp.3587~3596 (2007)[DOI]
  20. Lee, J. Y., "Characteristics of the ambient particulate PAHs at Seoul, a mega city of Northeast Asia in comparison with the characteristics of a background site", Atmospheric Research, 99(1), pp.50~56 (2011)[DOI]
  21. "Ambient air quality standards. GB 3095-2012" (2012)[URL]
  22. "Monthly Report of Air Quality" (2020)[URL]
  23. Mu, X., "An emission inventory of polycyclic aromatic hydrocarbons in China", EGU General Assembly Conference Abstracts (2015)
  24. Nisbet, I. C. T., "Toxic equivalency factors(TEFs)for polycyclic aromatic hydrocarbons(PAHs)", Regulatory Toxicology and Pharmacology, 16(3), pp.290~300 (1992)[DOI]
  25. "An Asian emission inventory of anthropogenic emission sources for the period 1980-2020" (2007)[URL]
  26. Seinfeld, J. H., "Atmospheric chemistry and physics : from air pollution to climate change" (2016), John Wiley & Sons
  27. Shin, S. M., "Seasonal variation and source apportionment of Oxygenated Polycyclic Aromatic Hydrocarbons(OPAHs)and Polycyclic Aromatic Hydrocarbons(PAHs)in PM2. 5 in Seoul, Korea", Atmospheric Environment, 272, pp.118937~ (2022)[DOI]
  28. Song, I. H., "Seasonal characteristics of PM1 in Seoul, Korea, measured using HR-ToF-Aerosol Mass Spectrometer in 2018", Atmospheric Environment, 266, pp.118717~ (2021)[DOI]
  29. "Office of the Federal Registration (OFR) Appendix A: priority pollutants" (1982)[URL]
  30. Vuong, Q. T., "Passive air sampling of halogenated polycyclic aromatic hydrocarbons in the largest industrial city in Korea : Spatial distributions and source identification", Journal of Hazardous Materials, 382, pp.121238~ (2020)[DOI]
  31. Wang, T., "Spatiotemporal distribution of atmospheric polycyclic aromatic hydrocarbon emissions during 2013–2017 in mainland China", Science of the Total Environment, 789, pp.148003~ (2021)[DOI]
  32. Wang, Z., "The seasonal variation, characteristics and secondary generation of PM2. 5 in Xi'an, China, especially during pollution events", Environmental Research, 212, pp.113388~ (2022)[DOI]

관련 논문AI추천

이 간행물의 다른 논문 (1건)