An optimization design study of producing transuranic nuclides in high flux reactor
2
조회
0
다운로드
1
인용
0
참고문헌
키워드
초록
Transuranic nuclides (such as 238Pu, 252Cf, 249Bk, etc.) have a wide range of application in industry, medicine, agriculture, and other fields. However, due to the complex conversion chain and remarkable fission losses in the process of transuranic nuclides production, the generation amounts are extremely low. High flux reactor with high neutron flux and flexible irradiation channels, is regarded as the promising candidate for producing transuranic nuclides. It is of great significance to increase the conversion ratio of transuranic nuclides, resulting in higher efficiency and better economy. In this paper, we perform an optimization design evaluation of producing transuranic nuclides in high flux reactor, which includes optimization design of irradiation target and influence study of reactor core loading. It is demonstrated that the production rate increases with appropriately determined target material and target structure. The target loading scheme in the irradiation channel also has a significant influence on the production of transuranic nuclides
Abstract
Transuranic nuclides (such as 238Pu, 252Cf, 249Bk, etc.) have a wide range of application in industry, medicine, agriculture, and other fields. However, due to the complex conversion chain and remarkable fission losses in the process of transuranic nuclides production, the generation amounts are extremely low. High flux reactor with high neutron flux and flexible irradiation channels, is regarded as the promising candidate for producing transuranic nuclides. It is of great significance to increase the conversion ratio of transuranic nuclides, resulting in higher efficiency and better economy. In this paper, we perform an optimization design evaluation of producing transuranic nuclides in high flux reactor, which includes optimization design of irradiation target and influence study of reactor core loading. It is demonstrated that the production rate increases with appropriately determined target material and target structure. The target loading scheme in the irradiation channel also has a significant influence on the production of transuranic nuclides
참고문헌 (10)
- C. Fry, "Discovery of isotopes of the transuranium elements with 93≤Z≤98", Atomic Data Nucl. Data Tables, 99, pp.96~114 (2013)
- P. B. Nuno, "Applications of research reactors", Encyclopedia of Nuclear Energy, 4, pp.8~25 (2021)
- R. C. Martin, "distribution and application of Californium-252neutron sources", Appl. Radiat. Isot, 53, pp.785~792 (2000)
- S. M. Robinson, "Production of Cf-252 and other transplutonium isotopes at Oak ridge national laboratory", Radiochim. Acta : Int. J. Chem. Aspects. Nucl. Sci. Technol, 108(9), pp.737~746 (2020)
- Y. A. Karelin, "RIRA reactor produced radionuclides", Appl. Radiat. Isot, 49(4), pp.299~304 (1998)
- R. B. Benjamin, "Design optimization methods for high-performance research reactor core design", Nucl. Eng. Des, 352, pp.110167~ (2019)
- P. K. Romano, "The OpenMC Monte Carlo particle transport code", Ann. Nucl. Energy, 51, pp.274~281 (2013)
- J. Li, "The NUIT code for nuclide inventory calculations", Ann. Nucl. Energy, 148, pp.107690~ (2020)
- H. Susan, "Increasing transcurium production efficiency through directed resonance shielding", Ann. Nucl. Energy, 60 (2013)
- Manual for Reactor Produced Radioisotopes, "IAEA", International Atomic Energy Agency, ~, pp.IAEA-TECDOC-1340 (2003)
