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The SPIZWURZ project – Experimental investigations and modeling of the behavior of hydrogen in zirconium alloys under long-term dry storage conditions

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In order to investigate the occurring processes during long-term dry storage of spent fuel assemblies, a joined project called SPIZWURZ, between the Karlsruhe Institute of Technology and the Gesellschaft für Anlagen-und Reaktorsicherheit (GRS), was started. Aim of the SPIZWURZ project is the determination and quantification of the influence of texture and elastic strain on diffusion and solubility of hydrogen in three different zirconium alloys used in western Europe during a long-term cooling transient (1 K/d) starting at 400 ◦C. The strain in the cladding of an irradiated spent fuel rod shall be measured. Models predicting the formation of radial oriented hydrides will be validated, improved, and implemented in the GRS fuel rod performance code TESPA-ROD. This paper describes the SPIZWURZ project and already obtained first results.

Abstract

In order to investigate the occurring processes during long-term dry storage of spent fuel assemblies, a joined project called SPIZWURZ, between the Karlsruhe Institute of Technology and the Gesellschaft für Anlagen-und Reaktorsicherheit (GRS), was started. Aim of the SPIZWURZ project is the determination and quantification of the influence of texture and elastic strain on diffusion and solubility of hydrogen in three different zirconium alloys used in western Europe during a long-term cooling transient (1 K/d) starting at 400 ◦C. The strain in the cladding of an irradiated spent fuel rod shall be measured. Models predicting the formation of radial oriented hydrides will be validated, improved, and implemented in the GRS fuel rod performance code TESPA-ROD. This paper describes the SPIZWURZ project and already obtained first results.

참고문헌 (10)

  1. ESK, "iskussionspapier zur verlangerten Zwischenlagerung bestrahlter Brennelemente und sonstiger Warme ¨ entwickelnder radioaktiver Abfalle" (2015), Entsorgungskommission
  2. S. Weick, "The SPIZWURZ Project with New Approaches for Experiments and Modelling Related to Long Term Dry Storage", TopFuel, Raleigh NC
  3. M. Grosse, "Quantitative determination of absorbed hydrogen in oxidised zircaloy by means of neutron radiography", Nucl. Instrum. Methods Phys. Res. A, 566, pp.739~745 (2006)[DOI]
  4. S. Weick, "The INCHAMEL facility – a new device for in-situ neutron investigations under defined temperatures with applicable mechanical load, submitted to", J. Phys. Conf
  5. T. Wiss, "Evolution of spent nuclear fuel in dry storage conditions for millennia and beyond", J. Nucl. Mater, 451, pp.198~ (2014)
  6. D. Prieur, "Elaboration de combustible `a base d’oxydes d’uranium et d’am´ericium : mod´elisation thermos-dynamique et propri´et´es des mat´eriaux", PhD, pp.2011
  7. G. Spykman, "Dry storage of spent nuclear fuel and high active waste in Germany-current situation and technical aspects on inventories integrity for a prolonged storage time", Nucl. Eng. Technol, 50(2), pp.313~ (2018)[DOI]
  8. F. Boldt, "Benchmark for the Simulation of Hydrogen Diffusion in Fuel Rod Claddings, Benchmark Specifications Version 2", ~ (2022)
  9. F. Boldt, "Implementation of Hydrogen Solid Solubility and pre-cipitation Threshold stresses in the fuel rod code TESPA-ROD", Nucl. Enging & Radiation Sci (2019), ASME[DOI]
  10. F. Boldt, "The SPIZWURZ Project –Progress and Benchmark Update", Proc., 27th Intern. QUENCH Workshop, Karlsruhe Institut für Technologie (KIT)

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