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Possibility of Curium as a Fuel for VVER-1200 Reactor

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초록

In this research, curium oxide (CmO2) is studied as fuel for VVER-1200 reactor to get an attention to its energy value and possibilities. For this purpose, CmO2 is used in fuel rods or integrated burnable absorber (IBA) rods with and without UO2 and then compared with the conventional fuel assembly of VVER-1200 reactor. It is burned to 60 GWd/t by using SRAC-2006 code and JENDL-4.0 data library. From these studies, it is found that CmO2 is competent like UO2 as a fuel due to higher fission cross-section of 243Cm and 245Cm isotopes and neutron capture cross-section of 244Cm and 246Cm isotopes. As a result, when some or all of the UO2 of fuel rods or IBA rods are replaced by CmO2, we get a similar k-inf like the reference even with lower enrichment UO2 fuels. These studies show that the use of CmO2 as IBA rods is more effective than the fuel rods considering the initially loaded amount, power peaking factor (PPF), fuel temperature and void coefficient, and the quality of spent fuel. From a detailed study, 3% CmO2 with inert material ZrO2 in IBA rods are recommended for the VVER-1200 reactor assembly from the once through concept.

Abstract

In this research, curium oxide (CmO2) is studied as fuel for VVER-1200 reactor to get an attention to its energy value and possibilities. For this purpose, CmO2 is used in fuel rods or integrated burnable absorber (IBA) rods with and without UO2 and then compared with the conventional fuel assembly of VVER-1200 reactor. It is burned to 60 GWd/t by using SRAC-2006 code and JENDL-4.0 data library. From these studies, it is found that CmO2 is competent like UO2 as a fuel due to higher fission cross-section of 243Cm and 245Cm isotopes and neutron capture cross-section of 244Cm and 246Cm isotopes. As a result, when some or all of the UO2 of fuel rods or IBA rods are replaced by CmO2, we get a similar k-inf like the reference even with lower enrichment UO2 fuels. These studies show that the use of CmO2 as IBA rods is more effective than the fuel rods considering the initially loaded amount, power peaking factor (PPF), fuel temperature and void coefficient, and the quality of spent fuel. From a detailed study, 3% CmO2 with inert material ZrO2 in IBA rods are recommended for the VVER-1200 reactor assembly from the once through concept.

참고문헌 (9)

  1. J.C. Posey, "Curium-244 isotopic power fuel: chemical recovery from commercial power reactor fuels", CONF-730602-1 4, ~ (1973)
  2. "Separations campaign (TRP) transmutation research program projects"[URL]
  3. T.S. Dikova, "Investigation the possibility of burning Cm a curium fuel reactor", J. Phys. Conf, pp.12048~ (2020)
  4. M. Osaka, "Analysis of curium in mixed oxide fuel irradiated in the experimental fast reactor joyo for the evaluation of its transmutation behavior", J. Nucl. Sci. Technol, 41(9), pp.907~914 (2004)[DOI]
  5. S. Pillon, "Aspects of fabrication of curium-based fuels and targets", J. Nucl. Mater, 320(1-2) (2003)
  6. Afroza Shelley, "Use of americium as a burnable absorber for VVER-1200 reactor", Nuclear Engineering and Technology, 53(8), pp.2454~2463 (2021), 한국원자력학회[DOI]
  7. SRAC2006: A Comprehensive Neutronics Calculation Code System, "K. Okumura", Japan Atomic Energy Agency, ~, pp.JAEA-Data (2007), Code 2007-004
  8. K. Shibta, "JENDL-4.0: a new library for nuclear science and engineering", J. Nucl. Sci. Technol, 48(1), pp.1~30 (2011)
  9. A. Sasahara, "Neutron and gamma ray source evaluation of LWR high burn-up UO2 and MOX spent fuels", J. Nucl. Sci. Technol, 41(4), pp.448~456 (2004)

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