Evaluation of particle-capturing ability of a hydrogel-based surface decontamination agent using simulated nuclear fallout particles
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Surface decontamination agents must effectively capture particle contaminants that have been deposited on surfaces. This ability is particularly important in scenarios involving nuclear fallout particles. In this technical note, the particle-capturing ability of a hydrogel, specifically, the polyvinyl alcohol-borax complex, was investigated as a potential decontamination agent for treating radioactively contaminated surface. For the assessment, simulated nuclear fallout particles, prepared by melting consolidation at 1200 ◦C followed by mechanical milling, were fixed on a stainless-steel substrate. The results demonstrated that the hydrogel effectively removed the simulated fallout particles from the surface. Even after only 1 min of contact time, the surface was left thoroughly clean, demonstrating the effectiveness of the polyvinyl alcohol-borax complex as a surface decontamination agent.
Abstract
Surface decontamination agents must effectively capture particle contaminants that have been deposited on surfaces. This ability is particularly important in scenarios involving nuclear fallout particles. In this technical note, the particle-capturing ability of a hydrogel, specifically, the polyvinyl alcohol-borax complex, was investigated as a potential decontamination agent for treating radioactively contaminated surface. For the assessment, simulated nuclear fallout particles, prepared by melting consolidation at 1200 ◦C followed by mechanical milling, were fixed on a stainless-steel substrate. The results demonstrated that the hydrogel effectively removed the simulated fallout particles from the surface. Even after only 1 min of contact time, the surface was left thoroughly clean, demonstrating the effectiveness of the polyvinyl alcohol-borax complex as a surface decontamination agent.
참고문헌 (28)
- K. -H. Schmidt, "Review on the progress in nuclear fission—experimental methods and theoretical descriptions", Rep. Prog. Phys, 81, pp.106301~ (2018)[DOI]
- N. Schunk, "Theory of nuclear fission", Prog. Part. Nucl. Phys, 125, pp.103963~ (2022)[DOI]
- E. A. C. Crouch, "Fission-product yields from neutron-induced fission", Atomic Data Nucl. Data Tables, 19, pp.417~532 (1977)[DOI]
- W. H. Langham, "Cs137 biospheric contamination from nuclear weapons tests", Health Phys, 2, pp.30~48 (1959)[DOI]
- O. Cheremisina, "Problems of protection of urban areas from radionuclides strontium-90 and caesium-137 after technological disasters", J. Ecol. Eng, 18, pp.97~103 (2017)[DOI]
- H. L. Beck, "Historical overview of atmospheric nuclear weapons testing and estimates of fallout in the continental United States", Health Phys, 82, pp.591~608 (2002)[DOI]
- M. Eisenbud, "Radioactive dust from nuclear detonations", Science, 117, pp.141~147 (1953)[DOI]
- S. R. Joshi, "Airborne radioactive materials and plants : a review", Sci. Total Environ, 24, pp.101~117 (1982)[DOI]
- A. Gossard, "Gels, coatings and foams for radioactive surface decontamination: state of the art and challenges for the nuclear industry", Prog. Nucl. Energy, 149, pp.104255~ (2022)[DOI]
- M. Endo, "Road surface washing system for decontaminating radioactive substances", 2014 IEEE, 2014, 1956~1961
- Y. Kameo, "Removal of metal oxide layers as a dry decontamination technique utilizing bead reaction and thermal quenching by dry ice blasting", J. Nucl. Sci. Technol, 43, pp.798~805 (2006)[DOI]
- Z. Nem´eth, "Comparative study of the corrosion and surface chemical effects of the decontamination technologies", J. Radioanal. Nucl. Chem, 286, pp.815~821 (2010)[DOI]
- H. M. Yang, "Polyvinyl alcohol-borate hydrogel containing magnetic adsorbent for surface decontamination", Ann. Nucl. Energy, 109, pp.359~364 (2017)[DOI]
- H. M. Yang, "Polymeric coatings for surface decontamination and ecofriendly volume reduction of radioactive waste after use", Prog. Nucl. Energy, 104, pp.67~74 (2018)[DOI]
- H. M. Yang, "Polyvinyl alcoholborate hydrogel containing Prussian blue for surface decontamination", J. Radioanal. Nucl. Chem, 316, pp.955~962 (2018)[DOI]
- H. M. Yang, "Enhanced surface decontamination of radioactive Cs by self-generated, strippable hydrogels based on reversible cross-linking", J. Hazard Mater, 362, pp.72~81 (2019)[DOI]
- H. M. Yang, "Poly(vinyl alcohol)-borax complex-based spray coating for the decontamination of radioactive Cs from wide-area surfaces", Chem. Eng. J, 402, pp.126299~ (2020)[DOI]
- H. M. Yang, "Surface decontamination of radioactive cesium by a reversibly cross-linkable hydrogel using poly(vinyl alcohol)and phenylboronic acid-grafted poly(methyl vinyl ether-alt-mono-sodium maleate)", Chemosphere, 339, pp.139617~ (2023)[DOI]
- Z. Y. He, "Study on the influencing factors in the process of surface strippable decontaminant", Coatings, 10, pp.649~ (2020)[DOI]
- G. Toader, "Water-based strippable coatings containing bentonite clay for heavy metal surface decontamination", Arab. J. Chem, 12, pp.4026~4034 (2019)[DOI]
- D. Pulpea, "Decontamination of radioactive hazardous materials by using novel biodegradable strippable coatings and new generation complexing agents", Chemosphere, 258, pp.127227~ (2020)[DOI]
- Technical Report for the Demonstration of Wide Area Radiological Decontamination and Mitigation Technologies for Building Structures and Vehicles, "R. James", ~, pp.EPA (2016), 600[DOI]
- T. Genda, "Iron-rich microstructure records of high temperature multi-component silicate melt behavior in nuclear fallout", J. Environ. Radioact, 237, pp.106700~ (2021)[DOI]
- P. H. Donohue, "Nuclear forensic applications involving high spatial resolution analysis of Trinitite cross-sections", J. Radioanal. Nucl. Chem, 306, pp.457~467 (2015)[DOI]
- M. M. A. Wannier, "Fallout melt debris and aerodynamically-shaped glasses in beach sands of Hiroshima Bay, Japan", Anthropocene, 25, pp.100196~ (2019)[DOI]
- N. Eby, "Trinitite-the atomic rock", Geol. Today, 26, pp.180~185 (2010)[DOI]
- C. A. Nizinski, "Production and characterization of synthetic urban nuclear melt glass", Nucl. Chem, 314, pp.2349~2355 (2017)[DOI]
- S. Sutou, "Black rain in Hiroshima: a critique to the Life Span Study of A-bomb survivors, basis of the linear no-threshold model", Gene Environ, 42, pp.1~ (2020)[DOI]
