고함량 Gd2O3 첨가 UO2 핵연료 소결체의 혼합 분말 입도에 따른 미세구조 영향 분석
Influence of Powder Particle Size on the Microstructure of UO2 Fuel Pellets with High Gd2O3 Content
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초록
The recent development of small modular reactors (SMRs) and the adoption of higher-enrichment fuels have intensified the need for advanced burnable absorbers to ensure effective reactivity control and extended fuel cycles. Among various designs, UO2 fuels with high Gd2O3 (gadolinium oxide) content provide notable benefits; in particular, they are compatible with established fabrication methods for burnable absorber fuels. However, achieving a homogeneous dispersion of Gd2O3 at high loading levels remains challenging, and the frequent occurrence of phase segregation and non-uniform microstructures can limit fuel reliability and performance. Overcoming these limitations requires an understanding of the powder characteristics and mixing behaviors during fabrication. In this study, we investigate the effects of the initial particle size and mixing method of UO2 and Gd2O3 powders on the microstructure and mixing homogeneity of high-Gd2O3-content fuels. The findings indicate that both the mixing method and the preparation state of the starting powders significantly affect the resulting microstructure and mixing uniformity.
Abstract
The recent development of small modular reactors (SMRs) and the adoption of higher-enrichment fuels have intensified the need for advanced burnable absorbers to ensure effective reactivity control and extended fuel cycles. Among various designs, UO2 fuels with high Gd2O3 (gadolinium oxide) content provide notable benefits; in particular, they are compatible with established fabrication methods for burnable absorber fuels. However, achieving a homogeneous dispersion of Gd2O3 at high loading levels remains challenging, and the frequent occurrence of phase segregation and non-uniform microstructures can limit fuel reliability and performance. Overcoming these limitations requires an understanding of the powder characteristics and mixing behaviors during fabrication. In this study, we investigate the effects of the initial particle size and mixing method of UO2 and Gd2O3 powders on the microstructure and mixing homogeneity of high-Gd2O3-content fuels. The findings indicate that both the mixing method and the preparation state of the starting powders significantly affect the resulting microstructure and mixing uniformity.
